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Origami is one of the simplest of art forms because the only materials needed are your hands and pieces of paper. Using only pieces of paper, an experienced paperfolder can make an almost limitless number of origami models.

You can purchase origami paper at most art supply stores. Origami paper comes in a variety of colors, patterns, sizes and textures. Most origami models can be folded using any type of origami paper, but sometimes the model that you are folding will dictate the type of paper that you will use. In general, you should use thin paper when folding a complex model that has many folds. Heavy paper should be used when folding a large-scale model.

Keep in mind that you do not really need to buy origami paper to make origami. You can use any paper available in your home - loose-leaf paper, typewriting paper, and even gift-wrapping paper. All you have to do is cut the paper into squares (or whatever shape is required by the model) and you are ready to fold.

Origami paper, often referred to as "kami" (Japanese for paper), is sold in prepackaged squares of various sizes ranging from 2.5 cm to 25 cm or more. It is commonly colored on one side and white on the other; however, dual coloured and patterned versions exist and can be used effectively for color-changed models. Origami paper weighs slightly less than copy paper, making it suitable for a wider range of models.

Normal copy paper with weights of 70–90 g/m2 can be used for simple folds, such as the crane and waterbomb. Heavier weight papers of (19-24&nb 100 g/m2 (approx. 25 lb) or more can be wet-folded. This technique allows for a more rounded sculpting of the model, which becomes rigid and sturdy when it is dry.

Foil-backed paper, just as its name implies, is a sheet of thin foil glued to a sheet of thin paper. Related to this is tissue foil, which is made by gluing a thin piece of tissue paper to kitchen aluminium foil. A second piece of tissue can be glued onto the reverse side to produce a tissue/foil/tissue sandwich. Foil-backed paper is available commercially, but not tissue foil; it must be handmade. Both types of foil materials are suitable for complex models.

Washi (和紙?) is the traditional origami paper used in Japan. Washi is generally tougher than ordinary paper made from wood pulp, and is used in many traditional arts. Washi is commonly made using fibres from the bark of the gampi tree, the mitsumata shrub (Edgeworthia papyrifera), or the paper mulberry but also can be made using bamboo, hemp, rice, and wheat.

Artisan papers such as unryu, lokta, hanji, gampi, kozo, saa, and abaca have long fibres and are often extremely strong. As these papers are floppy to start with, they are often backcoated or resized with methylcellulose or wheat paste before folding. Also, these papers are extremely thin and compressible, allowing for thin, narrowed limbs as in the case of insect models.

Paper money from various countries is also popular to create origami with; this is known variously as Dollar Origami, Orikane, and Money Origami.
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